The voice actresses called Alicia "Evilicia" after a few recording sessions when they realized she had to be hiding something dark behind her smile. This especially came to play during the recording for Episode 15 of The Natural when Alicia originally told Akari that she happened to gather people around her by chance, rather than the changed line of gathering people without realizing it. Alicia's voice actress realized that the original line made it sound like Alicia was talking down to Akari and convinced the director to change it. Alicia's evil side is played with in the picture dramas.
They're also convinced that Al has Aika wrapped around his finger and is manipulating her.
Awesome Music: Throughout all seasons. It makes one wonder why the makers go through such great lengths for a series that is clearly aimed at a niche audience.
The unexpectedly melancholic opening tune of Arietta.
Special note goes to Athena's song, "Barcarole", frequently acknowledged as in-universe Awesome Music.
The song that Alice sings during her promotional exam, "Lumis Eterne," with bonus points for being in Esperanto.
Big-Lipped Alligator Moment: Akari chasing down some runaway balls and rings from a circus group she suddenly decided to practice with in the 2nd story of season 1's episode 8.
Les Yay: The yuri fandom of the day went wild over Alicia and Akari having any scenes together. Their deep love and admiration of each other, as well as the fact that they share many intimate moments, made their Pseudo-Romantic Friendship very popular.
Memetic Mutation: Alicia's "Ara Ara"note Translated as "My My" interjection wouldn't be popularized until 14 years later, but it became a hallmark for characters of her Cool Big Sis/Onee-sama archetype.